The technique for recording Raman spectra in uranium compounds using a probe minispectrometer with a multielement radiation detector has been developed. A selective filter, which reflects exciting laser radiation and transmits Raman signals, has been used to suppress the exciting radiation. It is shown that the technique developed makes it possible to record Raman spectra from a small amount (~10–5 g) of sodium uranyl-acetate polycrystals in a wide spectral range for several seconds.