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요약정보
典型废塑料热解行为和动力学研究 / Study of pyrolysis behavior and kinetics of typical waste plastics
Resource Type
Academic Journal
Authors
尹凤福
;
庄虔晓
;
张超
;
孙启坤
;
YIN Fengfu
;
ZHUANG Qianxiao
;
ZHANG Chao
;
SUN Qikun
Source
弹性体 / China Elastomerics
. 30(6):19-23
Subject
混合塑料
共热解
活化能
动力学参数
热解机理
Language
Chinese
ISSN
1005-3174
Online Access
Find it @ DONGA
초록
对聚苯乙烯(PS)、丙烯腈-丁二烯-苯乙烯共聚物(ABS)单体及其与聚丙烯(PP)、聚氯乙烯(PVC)、聚乙烯(PE)的混合物进行了热重(TG)和差示扫描(DSC)实验,研究了PS和ABS单组分的热解特性和动力学参数,分析了PS和ABS对典型废旧塑料混合物(PP/PVC/PE)共热解行为的影响.结果表明,PS和ABS的热解反应为一步完成,剧烈热失重时间分别为3.4 min和4.8 min,PS的最大热解速率高于ABS,且ABS的热稳定性强于PS.对比两种混合物的实验结果可以发现,ABS与PS的加入使PP/PVC/PE混合物的残余质量增加,热解第二阶段最大速率降低.采用Kissinger法得到PS和ABS活化能为177.360 kJ/mol和188.566 kJ/mol,通过Criado法、Coast-Redfern法验证了PS和ABS的热解机理分别为随机成核随后生长的A 3/2和收缩圆柱体R2.
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