Two-dimensional plasmonic polarons in n-doped monolayer MoS2
- Resource Type
- Working Paper
- Authors
- Caruso, Fabio; Amsalem, Patrick; Ma, Jie; Aljarb, Areej; Schultz, Thorsten; Zacharias, Marios; Tung, Vincent; Koch, Norbert; Draxl, Claudia
- Source
- Phys. Rev. B 103, 205152 (2021)
- Subject
- Condensed Matter - Strongly Correlated Electrons
Condensed Matter - Materials Science
- Language
We report experimental and theoretical evidence of strong electron-plasmon interaction in n-doped single-layer MoS2. Angle-resolved photoemission spectroscopy (ARPES) measurements reveal the emergence of distinctive signatures of polaronic coupling in the electron spectral function. Calculations based on many-body perturbation theory illustrate that electronic coupling to two-dimensional (2D) carrier plasmons provides an exhaustive explanation of the experimental spectral features and their energies. These results constitute compelling evidence of the formation of plasmon-induced polaronic quasiparticles, suggesting that highly-doped transition-metal dichalcogenides may provide a new platform to explore strong-coupling phenomena between electrons and plasmons in 2D.