For Zn anodes of aqueous rechargeable zinc-ion batteries, the poor electrochemical performance causedby undesirable zinc dendritic formation and side reactions limit their practical application. Herein, a Zn2+redistributor is created to reduce dendrites growth by inserting a cellulose triacetate (CTA) film as aninterlayer between the zinc anode and the separator. The zinc dendritic formation and side reactionscan be suppressed by the CTA interlayer. Consequently, the Zn anode covered by CTA interlayer exhibitshighly reversible plating/stripping behavior with lifetime exceeding 2500 h and 600 h at current densitiesof 1 and 5 mA cm2, respectively. In particular, the electrochemical performance of the full cells is investigatedby using VO2 as the cathode and the CTA as interlayer. The Zn + CTA||VO2 full cells exhibit superiorperformance including high reversible capacity (490.2 mAh g1 at 0.2 A g1), excellent cycle performance(60.2% and 71.5% capacity retention after 5000 cycles at 5 A g1 and 10 A g1) and superior rate performance. This work demonstrates that designing a CTA interlayer is considered a cost-effective strategy tolight up the practical application of aqueous zinc-ion batteries.