The structural and magnetic properties of the single-phase pseudobinary ErFe Al compound, obtained under arc-melting conditions, have been investigated. Single crystal X-ray diffraction analysis revealed that this compound is stabilized with a hexagonal CeNi -type structure (space group P6 /mmc). The partial substitution of Fe by Al in this compound occurring at all the metallic sites is reflected in the decrease of the Curie temperature Tc. Magnetization curves (2-450 K; 0-5 T) indicate a ferrimagnetic ordering with four magnetic phases induced by competitional interactions between magnetic moments of both Er and Fe. The magnetocaloric effect has been estimated from the magnetic isotherms. The relative cooling power (RCP) value indicates relatively promising magnetic refrigerant material. [ABSTRACT FROM AUTHOR]